4.7 Article

A novel route to improve methane aromatization by using a simple composite catalyst

Journal

CHEMICAL COMMUNICATIONS
Volume 54, Issue 73, Pages 10343-10346

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/c8cc05059g

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Funding

  1. National Natural Science Foundation of China [21606249, 21501186]
  2. Strategic Priority Research Program'' of the Chinese Academy of Sciences [XDB17020100]
  3. Chinese Academy of Sciences [Y57201190V]
  4. Director Innovation Fund of Key Laboratory of Biofuels

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A simple composite catalyst was proposed for the first time for methane aromatization, consisting of Mo/HZSM-5 for methane dehydroaromatization (MDA) and Ce0.9Gd0.1Oy (CGO) for hydrogen combustion. The redox properties of CGO and its high selectivity towards hydrogen oxidation enable an efficient periodic MDA reaction/regeneration process, leading to improved methane aromatization.

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