Journal
CHEMICAL COMMUNICATIONS
Volume 50, Issue 23, Pages 3048-3051Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc49059a
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Funding
- Major Basic Research Development Program [2011CB808706]
- National Natural Science Foundation of China [21272251, 21121062, 21032007]
- Chinese Academy of Sciences
- Technology Commission of Shanghai Municipality
- Croucher Foundation of Hong Kong
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A new strategy for the construction of a C=C-CF3 subunit has been developed via CuBr-catalyzed domino cyclization-trifluoromethylation of homopropargyl amines with Umemoto's reagent. 4-Trifluoromethyl-2,3- dihydro-pyrroliums were produced in high yields. The usefulness of these products has been demonstrated by the transformation of them into various other trifluoromethylated molecules.
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