Journal
CHEMICAL COMMUNICATIONS
Volume 50, Issue 31, Pages 4047-4049Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc49684h
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Funding
- National Basic Research Program of China [2012CB821706, 2013CB834803]
- National Natural Science Foundation of China [91222202, 21171114, 21101103, 21371113]
- Natural Science Foundation of Guangdong Province [S201140004334]
- Shantou University
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A Mn-based rod metal-organic framework (MOF), ROD-6, with a new lrk net is synthesized. It represents an unusual type of MOF topology containing both a 1-periodic secondary building unit (rod SBU) and a polytopic linker (here 1,3,6,8-tetrakis(p-benzoic acid) pyrene), and also exhibits high stability (up to 485 degrees C) and unusual CO2 uptake behaviour and selectivity despite the lack of strong interacting sites, demonstrated by the low and increasing heat of adsorption.
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