Journal
CHEMICAL COMMUNICATIONS
Volume 50, Issue 93, Pages 14670-14673Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cc05563b
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- Compagnia di San Paolo and Universita di Torino (PHOTORECARB project)
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The effect of a local proton source on the activity of a bromotricarbonyl Mn redox catalyst for CO2 reduction has been investigated. The electrochemical behaviour of the novel complex [fac-Mn(dhbpy)(CO)(3)Br] (dhbpy = 4-phenyl-6-(1,3-dihydroxybenzen-2-yl) 2,2'-bipyridine), containing two acidic OH groups in the proximity of the metal centre, under a CO2 atmosphere showed a sustained catalysis in homogeneous solution even in the absence of Bronsted acids.
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