Journal
CHEMICAL COMMUNICATIONS
Volume 50, Issue 56, Pages 7521-7523Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cc02768j
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Funding
- Nature National Science Foundation of China [21172106, 21074054, 21372114]
- National Basic Research Program of China [2010CB923303]
- Research Fund for the Doctoral Program of Higher Education of China [20120091110010]
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An effective approach to C1-difluoromethylated tetrahydroisoquinoline derivatives has been developed through C-H functionalization of tertiary amines by visible-light photoredox catalysis. This method uses stable, easily obtained alpha,alpha-difluorinated gem-diol as the CF2 source. The corresponding products were obtained in moderate to high yields at ambient temperature.
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