Journal
CHEMICAL COMMUNICATIONS
Volume 50, Issue 71, Pages 10251-10254Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cc04020a
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Funding
- NSFC [21102013, 51173065]
- Dalian Committee of Science and Technology [2011J21DW001]
- SRF for ROCS-SEM [201001438, 201001439]
- Fundamental Funds for the Central Universities [DUT11LK20]
- RFDP [20090041120017]
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Two novel asymmetrical push-pull small molecules have been synthesized successfully, consisting of triphenylamine and diketopyrrolopyrrole as a fundamental dipolar D-pi-A structure with ethynylbenzene as the pi-bridge. TPATDPPCN end-capped with cyanophenyl exhibits a low optical band gap of 1.65 eV, and an impressive PCE of 5.94% has been achieved.
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