Journal
CHEMICAL COMMUNICATIONS
Volume 49, Issue 63, Pages 7031-7033Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc42937g
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Funding
- Hong Kong Research Grants Council [PolyU5017-07P, SEG_PolyU01]
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Rh(III)-catalyzed aromatic C-H amination of acetophenone o-methyloximes with primary N-chloroalkylamines was developed, and the arylamine products were obtained in up to 92% yield. The reaction probably involves rate-limiting electrophilic C-H bond cleavage (k(H)/k(D) = 2).
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