Journal
CHEMICAL COMMUNICATIONS
Volume 49, Issue 80, Pages 9116-9118Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc45063e
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Funding
- EPSRC [EP/K021435/1, EP/F019327/2, EP/F019327/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/K021435/1, EP/F019327/1, EP/F019327/2] Funding Source: researchfish
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To what extent can a heterometallic chain of transition metal ions generate an asymmetric current-voltage response? Density functional theory suggests that the answer depends very much on the symmetry of the dominant conduction channel: pi channels are more localised and hence afford higher rectification ratios.
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