Journal
CHEMICAL COMMUNICATIONS
Volume 49, Issue 15, Pages 1542-1544Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2cc38165f
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Funding
- National Natural Science Foundation of China [21073086, 20833003]
- National Basic Research Program [2011CB808501]
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Density functional theory investigations reveal that a cavitand with an introverted aldehyde group not only provides the host-guest interaction for preorganizing the substrate and stabilizing the hemiaminal intermediate, but also acts as an acid/base catalyst in the subsequent dehydration step in its reaction with a primary amine.
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