Journal
CHEMICAL COMMUNICATIONS
Volume 49, Issue 36, Pages 3787-3789Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc41301b
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Funding
- Natural Science Foundation of China [NSFC 20473016, 20673018]
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Strongly adsorbed N atoms inhibit the ammonia decomposition reaction rate. Plasma-driven catalysis can solve this problem and increase the ammonia conversion from 7.8% to 99.9%. (NH3)-N-15 isotope tracing and optical emission spectroscopy show that gas-phase active species (NH3*, NH center dot) in the plasma zone facilitate the desorption step by an Eley-Rideal (E-R) interaction.
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