Journal
CHEMICAL COMMUNICATIONS
Volume 49, Issue 42, Pages 4743-4745Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc39008j
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Funding
- National Science Council of Taiwan
- Academia Sinica
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The first di-protonated [FeFe] hydrogenase model relevant to key intermediates in catalytic hydrogen production is reported. The complex bearing the S-proton and Fe-hydride is structurally and spectroscopically characterized as well as studied by DFT calculations. The results show that the thiolate sulfur can accept protons during the catalytic routes.
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