Journal
CHEMICAL COMMUNICATIONS
Volume 49, Issue 22, Pages 2192-2194Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc38009b
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Funding
- Cambridge Overseas Trust
- ERC
- Engineering and Physical Sciences Research Council [EP/K004042/1] Funding Source: researchfish
- EPSRC [EP/K004042/1] Funding Source: UKRI
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This paper presents a novel method and rationale for utilizing carbonized MOFs for sulphur loading to fabricate cathode structures for lithium-sulphur batteries. Unique carbon materials with differing hierarchical pore structures were synthesized from four types of zinc-containing metal-organic frameworks (MOFs). It is found that cathode materials made from MOFs-derived carbons with highermesopore (2-50 nm) volumes exhibit increased initial discharge capacities, whereas carbons with higher micropore (<2 nm) volumes lead to cathode materials with better cycle stability.
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