Journal
CHEMICAL COMMUNICATIONS
Volume 49, Issue 28, Pages 2909-2911Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc40516h
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Funding
- Knowledge Innovation Program of the Chinese Academy of Sciences [KJCX2-EW-H01]
- National Science Foundation of China [21003125, 21073190]
- National Science Foundation of Fujian Province [2010J05040, 2010J01057]
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An unprecedented 3-D SHG-active metal-organic framework (MOF) of silver(I), Ag-Amidn (1) (HAmidn: 2-amino-4,5-imidazole-dicarbonitrile), has been successfully prepared by employing the new single ligand. The cooperative coordination of the imidazole and carbonitrile N atoms leads to the chiral triple helices accounting for the noncentrosymmetric space group, which are linked together to form a rare 10(3) topological structure. Ag-Amidn (1) with high thermal stability and insolubility may be considered as a potential second-order NLO material.
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