Journal
CHEMICAL COMMUNICATIONS
Volume 48, Issue 9, Pages 1287-1289Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2cc16221k
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Funding
- University of Ottawa
- Canada Foundation for Innovation (CFI)
- FFCR
- NSERC
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A high-spin tridecanuclear Ni-II cluster, [Ni-II (13)(N-3)(18)(dpo)(4)(Hdpo)(2)(H(2)hpo)(4)(H2O)(MeOH)] [Ni-II (13)(N-3)(18)(dpo)(4)(Hdpo)(2)(H(2)hpo)(4)(H2O)(2)] (1) (Hdpo = 1-(dimethylamino) propan-2-one oxime and H(2)hpo = 1-(hydroxyamino) propan-2-one oxime) with a purely azido-bridged core, is reported with dominant ferromagnetic coupling between Ni-II ions. The latter molecule exhibits a unique planar core topology with the largest N-3 : Ni-II ratio reported to date.
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