Journal
CHEMICAL COMMUNICATIONS
Volume 48, Issue 11, Pages 1698-1700Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2cc16832d
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Funding
- National Natural Science Foundation of China [21032003, 20872140]
- National Basic Research Program of China [2010CB833300]
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Asymmetric hydrogenolysis of racemic tertiary alcohols, 3-substituted 3-hydroxyisoindolin-1-ones, was developed using chiral phosphoric acid as catalyst and a Hantzsch ester as the hydrogen source with up to 95% ee. The reaction process of this asymmetric transfer hydrogenation may occur directly through the acyliminium ion intermediate.
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