Journal
CHEMICAL COMMUNICATIONS
Volume 48, Issue 80, Pages 9995-9997Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2cc34622b
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Funding
- U.S. Department of Energy [DOE DE-SC0001015, DE-FC36-07GO17033]
- National Science Foundation [NSF CBET-0930079]
- Welch Foundation [A-1725]
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A multi-functional MOF PCN-124 was constructed from Cu paddlewheel motifs and a judiciously designed novel ligand bearing carboxylate, pyridine, and amide groups. PCN-124 exhibits selective adsorption of CO2 over CH4 and excellent catalytic activity in a tandem one-pot deacetalization-Knoevenagel condensation reaction as a cooperative catalyst.
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