Journal
CHEMICAL COMMUNICATIONS
Volume 48, Issue 56, Pages 7025-7027Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2cc17593b
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Funding
- Major State Basic Research Development Programs [2011CB808704]
- NSFC [20931004]
- Science Foundation of Innovative Research Team of NSFC [20721002]
- Fundamental Research Funds for the Central Universities [1114020501]
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Two mesoporous and flexible acylamide-functionalized rht-type MOFs exhibit not only high excess unsaturation CO2 uptake (157 wt%) at 20 bar and 273 K, but also good selectivity of CO2/CH4 (8.6) and CO2/N-2 (34.3). The advantages of acylamide groups for CO2 capture have been further confirmed by GCMC and first-principles calculations.
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