Journal
CHEMICAL COMMUNICATIONS
Volume 47, Issue 47, Pages 12706-12708Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1cc15946a
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Funding
- National Natural Science Foundation of China [21072020]
- Beijing Institute of Technology [2011CX01008, 2011CX03037]
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An efficient highly diastereo- and enantioselective direct Michael addition of nitroalkanes to nitroalkenes catalyzed by chiral squaramide catalyst has been developed. This organocatalytic reaction with a low catalyst loading (2 mol%) proceeded well to afford synthetically useful 1,3-dinitro compounds in high yields with high diastereoselectivities (up to 95:5 dr) and excellent enantioselectivities (up to 97% ee).
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