Journal
CHEMICAL COMMUNICATIONS
Volume 47, Issue 42, Pages 11745-11747Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1cc15501f
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Funding
- NSF
- Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-FG02-07ER15909]
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The catalytic water-oxidation activity of Wilkinson's iridium acetate trimer (1) has been characterized electrochemically and by using chemical oxidants. We show that 1 can function as an operationally homogeneous water-oxidation catalyst when driven with sodium periodate as a primary oxidant, but rapidly decomposes using Ce(IV) as a primary oxidant.
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