Journal
CHEMICAL COMMUNICATIONS
Volume 47, Issue 33, Pages 9345-9347Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1cc12391b
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Funding
- National Natural Science Foundation of China [21006068]
- Seed Foundation of Tianjin University [60303002]
- Program for New Century Excellent Talents in University
- Program of Introducing Talents of Discipline to Universities [B06006]
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This communication describes the design of bifunctional VOx/TS-1 catalysts with enhanced redox and acidic character via doping SO42- and PO43- for selective oxidation of methanol to dimethoxymethane. Redox sites enable the production of formaldehyde, while acidic sites favor the condensation of formaldehyde to DMM.
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