Journal
CHEMICAL COMMUNICATIONS
Volume 47, Issue 47, Pages 12607-12609Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1cc15071e
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Funding
- Army Research Office [W911NF-09-1-0426]
- UNC EFRC: Solar Fuels and Next Generation Photovoltaics, an Energy Frontier Research Center
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001011]
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Electrocatalytic reduction of CO2 by [Ru(tpy)(bpy)(solvent)](2+) (tpy = 2,2':6',2 ''- terpyridine, bpy = 2,2'-bipyridine) and its structural analogs is initiated by sequential 1e(-) reductions at the tpy and bpy ligands followed by rate limiting CO2 addition to give a metallocarboxylate intermediate. It undergoes further reduction and loss of CO.
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