Journal
CHEMICAL COMMUNICATIONS
Volume 46, Issue 48, Pages 9215-9217Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0cc03399e
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Funding
- German Business Foundation
- NSF [CHE-0840513]
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The first asymmetric total synthesis of fumimycin was accomplished. As a key step, a 1,2-addition of methyl Grignard reagents to ketimines with quinine as additive was employed. The absolute configuration of (+)-fumimycin was determined by CD-spectroscopy combined with time-dependent density functional calculations.
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