Journal
CHEMICAL COMMUNICATIONS
Volume 46, Issue 45, Pages 8621-8623Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0cc03190a
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Funding
- U.S. Department of Energy-Basic Energy Sciences [DE-FG02-07ER15896]
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Oxygen reduction reaction (ORR) over a carbonaceous catalyst (1) with a phosphinate (>P(=O)OH) moiety was explored computationally. Under the acidic environment of a fuel cell, 1 could be active for ORR and be converted to 2 with a >P(OH)(2) moiety. An edge phosphinate could be active for both 2- and 4-electron ORR.
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