Journal
CHEMICAL COMMUNICATIONS
Volume 46, Issue 29, Pages 5319-5321Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0cc00452a
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Funding
- NSF of China [20832005]
- National Basic Research Program (973 Program) of China [2010CB833200]
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Methyl tetramate derivative 6 has been developed as a new building block for the flexible and racemization-free synthesis of methyl 5-benzyl-3-methyltetramate via alkylation, and used in the first asymmetric synthesis of palau'imide (1). This allowed the establishment of the hitherto unknown stereochemistry at the C-20 of palau'imide as S.
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