Journal
CHEMICAL COMMUNICATIONS
Volume 46, Issue 45, Pages 8507-8525Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0cc02780d
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Funding
- Ministry of Education, Culture, Sports, Science, and Technology (MEXT), Japan
- Scientific Research-Flanders (FWO)
- Institute of Promotion of Innovation by Science and Technology in Flanders
- Belgian Federal Science Policy Office [IAP-6/27]
- JSPS
- FWO
- HIT
- Ministry of Education of P. R. China
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At the liquid/graphite interface triangular and rhombic phenylene-ethynylene macrocycles substituted by alkyl chains self-assemble to form porous two-dimensional (2D) molecular networks of honeycomb and Kagome types, respectively, or close-packed non-porous structures via alkyl chain interdigitation as the directional intermolecular linkages. Factors that affect the formation of the 2D molecular networks, such as alkyl chain length, solvent, solute concentration, and co-adsorption of guest molecules, were elucidated through a systematic study. For the porous networks, various molecules and molecular clusters were adsorbed in the pores reflecting the size and shape complementarity, exploring a new field of 2D host-guest chemistry.
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