Journal
CHEMICAL COMMUNICATIONS
Volume 46, Issue 25, Pages 4625-4626Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0cc00360c
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Funding
- Deutsche Forschungsgemeinshaft [DFG GS 13/2-1]
- Japan Society for Promotion of Science [FY2009 JSPS]
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NMR studies of (13)C/(12)C isotopic patterns in Cu(III) intermediates and reaction products together with DFT calculations of possible reaction pathways indicate an intermolecular S(N)2 like substitution mechanism for ligand exchange reactions in square planar Cu(III) complexes, which is proposed to be slow compared to reductive elimination at synthetic conditions.
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