Journal
CHEMICAL COMMUNICATIONS
Volume -, Issue 19, Pages 2652-2654Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/b901135h
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Funding
- Hydrogen Program of the Department of Energy [DE-FG36-05GO15040]
- National Science Foundation [DMR05-20415]
- NNIN (National Nanofabrication Infrastructure Network)
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CoF3 aqueous solution was used to modify the surface of Ti-doped iron oxide thin film photoanodes to negatively shift the flat-band potential and allow photogenerated electrons to directly reduce water to hydrogen without an external bias; the zero bias performance was further improved by the use of glucose (a biomass analog) to bypass the relatively slow oxygen evolution reaction to provide a source of electrons to rapidly consume photogenerated holes.
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