4.6 Article

Quantum spin liquid: The Heisenberg antiferromagnet on the three-dimensional pyrochlore lattice

Journal

PHYSICAL REVIEW B
Volume 61, Issue 2, Pages 1149-1159

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.61.1149

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We calculate the correlation functions of the S=1/2 Heisenberg antiferromagnet on the three-dimensional pyrochlore lattice. We use a perturbative expansion in terms of spin blocks. This method is self-controlled by the extracted correlation length. We find that the ground state is a spin-liquid state: the spin-spin correlation functions decay exponentially with distance and the correlation length never exceeds the interatomic distance, even at T=0. The static structure factor becomes dispersive, indicating a selection of modes by thermal and quantum fluctuations. We also calculate the magnetic neutron diffraction cross section in two planes of the reciprocal space and we find a very good agreement with neutron experiments performed on Y(Sc)Mn-2 and CsNiCrF6.

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