Journal
CHEMICAL COMMUNICATIONS
Volume -, Issue 36, Pages 4309-4311Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/b807529h
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Lewis bases such as Ph(3)P = O and HMPA catalyze the 1,4-reduction of alpha,beta-unsaturated ketones with trichlorosilane, and because the 1,2-reduction of aldehydes scarcely proceeded under the conditions, one-pot reductive aldol reactions with aldehydes were successfully achieved; preliminary studies using a chiral Lewis base revealed a high potential for enantioselective catalysis.
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