Journal
CHEMICAL COMMUNICATIONS
Volume -, Issue 45, Pages 5883-5895Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/b810394a
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Funding
- National Institute of Health [GM-029028, CA-019033, GM-081253]
- NATIONAL CANCER INSTITUTE [R01CA019033] Funding Source: NIH RePORTER
- NATIONAL INSTITUTE OF GENERAL MEDICAL SCIENCES [P41GM081253, R01GM029028] Funding Source: NIH RePORTER
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Efficient construction of architecturally complex natural and unnatural products is the hallmark of organic chemistry. Anion relay chemistry (ARC) - a multi-component coupling protocol - has the potential to provide the chemist with a powerful synthetic tactic, enabling efficient, rapid elaboration of structurally complex scaffolds in a single operation with precise stereochemical control. The ARC tactic can be subdivided into two main classes, comprising the relay of negative charge either through bonds or through space, the latter with aid of a transfer agent. This review will present the current state of through-space anion relay, in conjunction with examples of natural and unnatural product syntheses that illustrate the utility of this synthetic method.
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