Journal
JOURNAL OF CRYSTAL GROWTH
Volume 208, Issue 1-4, Pages 416-422Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/S0022-0248(99)00468-6
Keywords
diamond-like quaternary compounds; synthesis; gradient freezing; melting point; lattice constant; crystal structure; optical band gap
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We have investigated the synthesis from the melts of Cu-III-IV-VI4 and Cu-2-II-IV-VI4 quaternary compounds (II = Zn, Cd, III = Ga, In; IV = Ge, Sn: VI = Se). Among these compounds. the single phases were obtained, except for CuGaSnSe4 and CuInSnSe4, and their melting points were determined using the differential thermal analysis. These crystal structures, and primitive optical and electrical properties of single crystals grown by the horizontal gradient freezing method from the melts, have been characterized. The CuGaGeSe4, CuInGeSe4, Cu2ZnSnSe4 and Cu2CdGeSe4 compounds are found to have band gaps suitable for optimum conversion efficiency for solar cells(1.2-1.5 eV). (C) 2000 Elsevier Science B.V. All rights reserved.
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