Journal
CHEMCATCHEM
Volume 6, Issue 8, Pages 2315-2321Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cctc.201402195
Keywords
layered compounds; palladium; photochemistry; reduction; self-assembly
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Funding
- National Environment Agency, Singapore under the Environment Technology Research Programme (ETRP) [ETRP 1002 103]
- Singapore National Research Foundation (NRF) through the Singapore-Berkeley Research Initiative for Sustainable Energy (SinBeRISE) CREATE Programme
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A self-assembly of carbon nitride (C3N4) and layered double hydroxide (LDH) was constructed by electrostatic interaction. The pristine nitrate-intercalated Mg-Al-LDH is turned to carbonate LDH through anion exchange during the photoreduction of CO2 in aqueous solution. The carbonate anions enriched in the interlayer of LDH exhibit a remarkably high reduction efficiency to CH4 in the presence of a C3N4 photoabsorber and Pd cocatalyst.
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