Journal
CHEMCATCHEM
Volume 6, Issue 3, Pages 713-718Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cctc.201301072
Keywords
ethylene; methanol; propylene; toluene; para-xylene
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Light olefins and para-xylene were produced with high selectivity in the reaction of toluene with methanol over a modified HZSM-5 catalyst. Ordered mesoporous structure and weaker acidic sites led to significant contribution to the selectivity toward para-xylene. By means of a single-pulse reaction and the temperature-programmed surface reaction, it was confirmed that the presence of toluene and as-produced xylene shortened the reaction induction period and reduced the formation temperature of ethylene and propylene, which was beneficial to improve the selectivity toward light olefins, particularly ethylene.
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