Journal
PHYSICAL REVIEW B
Volume 65, Issue 9, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.65.092401
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We study local lattice fluctuations in La1-xCaxMnO3(0.45less than or equal toxless than or equal to0.76)by means of inelastic light scattering. Fluctuation effects are especially strong in the intensity variation of Jahn-Teller mode at 480 cm(-1) around commensurate doping xapproximate to0.5. The linewidth of the Jahn-Teller mode shows a minimum at x=0.50 indicating long-range lattice and charge commensuration at low temperatures. The electron-phonon interaction is fundamentally changed at the transition to the charge-ordered (CO) state as evidenced by sign and magnitude changes in the Fano parameter. Temperature-dependent data show enhanced fluctuations persisting up to temperatures of at least 2 T-co for xapproximate to0.50.
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