Journal
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
Volume 4, Issue 11, Pages 2246-2250Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/b102700j
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This paper examines the temporal evolution of an electron in a photosynthetic reaction center. A model based on self-consistent quantum-mechanical equations is suggested to describe the picosecond transfer of an electron from an excited primary donor, the excited bacteriochlorophyll dimer (P*), to bacteriopheophytin ( H). This transfer is shown to have an oscillation behavior. The results obtained offer an explanation for oscillations in the emission kinetics of the primary donor excited state.
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