Journal
REACTION KINETICS AND CATALYSIS LETTERS
Volume 78, Issue 1, Pages 11-18Publisher
SPRINGER
DOI: 10.1023/A:1022593211955
Keywords
spillover hydrogen; hydrodechlorination; hydrogenation; nickel/silica
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Spillover hydrogen has been shown to contribute to gas phase aromatic hydrodechlorination and hydrogenation over Ni/SiO2 + SiO2 physical mixtures. The reaction rates (per unit mass Ni) are enhanced by extending the Ni/SiO2-SiO2 interface; a non-contiguous combination does not deliver any beneficial effect. The physical mixtures exhibited different selectivity trends for the conversion of 1,3,5-trichlorobenzene and served to prolong productive catalyst lifetime by inhibiting coke formation.
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