Journal
CHEMICAL ENGINEERING SCIENCE
Volume 58, Issue 2, Pages 269-273Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/S0009-2509(02)00518-3
Keywords
gas hydrate; structure-H; gases; phase equilibria; stability; solutions
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The four-phase coexistence curves for the structure-H hydrates of methylcyclohexane and cis-1,2-dimethylcyclohexane in the presence of methane are measured in the temperature range 274.09-288.29 K and pressure range 1.42-8.89 MPa. Very large pressure reductions from the pure methane hydrate are observed by forming structure-H hydrates. The present investigation on the trans-1,2-dimethylcyclohexane system reveals that the limit of the largest-cage occupancy for the structure-H hydrate is laid between the 1,2-dimethylcyclohexane stereo-isomers. (C) 2002 Elsevier Science Ltd. All rights reserved.
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