Journal
CATALYSIS LETTERS
Volume 134, Issue 1-2, Pages 155-161Publisher
SPRINGER
DOI: 10.1007/s10562-009-0227-1
Keywords
Metalloporphyrin; Cobalt acetate; co-Catalysis; p-Toluic acid; Oxidation; Terephthalic acid
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Funding
- National Natural Science Foundation of China [CN J0830415]
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The aerobic oxidation of p-toluic acid to terephthalic acid over tetra(p-chlorophenylporphinato)manganese (T(p-Cl)PPMnCl)/cobalt acetate was reported for the first time. The co-catalysis of T(p-Cl)PPMnCl/Co(OAc)(2) was also studied. The studies indicated that the PTA oxidation was influenced by the catalyst composition, catalyst concentrations and reaction conditions. A preliminary mechanism of this co-catalyzed oxidation reaction was proposed based on experimental observations.
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