Journal
CATALYSIS LETTERS
Volume 127, Issue 3-4, Pages 334-338Publisher
SPRINGER
DOI: 10.1007/s10562-008-9684-1
Keywords
Hydrogenation; Alkyne; Size effect; Shape effect; Pd-nanoparticle; AOT; CTAB
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Funding
- EPFL-CIME
- Swiss National Science Foundation
- Commission for Technology and Innovation (CTI)
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Palladium nanohexagons were prepared using a seed-mediated method. Their catalytic performance in 2-methyl-3-butyn-2-ol hydrogenation was compared to the one of monodispersed Pd nanospheres. Quantitative correlations between initial turnover frequencies (TOFs) and nanoparticle surface compositions showed independence of TOFs calculated per atoms on Pd(111) facets on particle size and shape.
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