Journal
CATALYSIS COMMUNICATIONS
Volume 22, Issue -, Pages 68-73Publisher
ELSEVIER
DOI: 10.1016/j.catcom.2012.02.012
Keywords
Hydrogen production; SMSI; Methanol reforming; Fuel processing; Microchannel reactor
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Funding
- DICP 100-Talent Program
- Natural Science Foundation of Liaoning Province [201102219]
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A series of NiZnAl catalysts have been developed for the hydrogen production by methanol steam reforming within microchannel reactor. These catalysts were characterized by N-2 adsorption-desorption, X-ray diffraction, H-2-TPR and pulse H-2-chemisorption. Our results show that the coexistence of Ni and Zn in bimetallic catalysts results in superior catalytic performance for hydrogen production compared with monometallic catalysts, despite the fact the former possesses the lower surface area. The difference between the catalytic performances could mainly be attributed to the Ni promotion effect associated with SMSI-like geometric effects and interpreted by a hypothesized encapsulation model corroborated by the characterizations. (C) 2012 Elsevier B.V. All rights reserved.
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