Journal
CATALYSIS COMMUNICATIONS
Volume 12, Issue 15, Pages 1405-1409Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.catcom.2011.05.007
Keywords
Catalytic hydrodechlorination; of 2,4-dichlorophenol; Supported Pd catalyst; Activated carbon; Mesoporous carbon
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Funding
- Natural Science Foundation of China [20877039]
- Program of New Century Excellent Talents in University [NECT-08-0277]
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Supported Pd catalysts on ordered mesoporous carbon (OMC) and activated carbon (AC) were prepared and their catalytic behavior for the liquid phase catalytic hydrodechlorination (HOC) of 2,4-dichlorophenol was investigated. In comparison with Pd/AC, Pd particles of Pd/OMC were effectively confined in the mesopores of OMC, resulting in high Pd dispersion and Pd(2+) content. Accordingly, Pd/OMC exhibited higher catalytic activity than Pd/AC. Moreover, increasing catalyst reduction temperature lowered the catalytic activities and favored stepwise HDC of 2,4-dichlorophenol. (C) 2011 Elsevier B.V. All rights reserved.
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