Journal
JOURNAL OF BIOLOGICAL PHYSICS
Volume 31, Issue 2, Pages 145-159Publisher
SPRINGER
DOI: 10.1007/s10867-005-5109-1
Keywords
charge oscillation; hopping; quinone; Schrodinger equation; superexchange
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A dynamical theory has been developed for primary separation of charges in the course of photosynthesis. The theory deals with both hopping and superexchange transfer mechanisms. Dynamics of electron transfer from dimeric bacteriochlorophyll to quinone has been calculated. The results obtained agree with experimental data and provide a unified explanation of both the hierarchy of the transfer time in the photosynthetic reaction center and the phenomenon of coherent oscillations accompanying the transfer process.
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