Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 11, Issue 1, Pages 112-119Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.200400540
Keywords
cyclic voltammetry; flavins; redox catalysis; redox chemistry
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Eight different flavin derivatives have been synthesized and the electronic effects of substituents in various positions on the flavin redox chemistry were investigated. The redox potentials of the flavins, determined by cyclic voltammetry, correlated with their efficiency as catalysts in the H2O2 oxidation of methyl p-tolyl sulfide. Introduction of electron-withdrawing groups increased the stability of the reduced catalyst precursor.
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