Journal
CARBON
Volume 43, Issue 3, Pages 541-549Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.carbon.2004.10.016
Keywords
activated carbon; adsorption; gas storage
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A homogeneous, isotropic porous matrix of activated carbon inside a portable steel cylinder is considered as the adsorption bed for natural gas (NG) which is idealized as pure methane for the purpose of simulation. The heat and fluid flow inside the porous adsorption bed are modeled using a volume averaging technique and Darcy-Brinkman formulation. The effective thermal conductivity of the activated-carbon-methane system is calculated as a function of uptake according to the Luikov model. Heat generation due to the exothermic process of adsorption is considered. The governing equations are solved using an implicit finite volume method for the given boundary conditions. Three different models of adsorption are considered, namely (i) a no-flow model, (ii) flow model with uniform adsorption and (iii) a flow model with local adsorption. For each of these models, transient temperature profiles in the adsorption bed during the charging process are obtained, and the corresponding mass adsorption potentials are calculated. Parametric studies are performed to investigate the effects of gas inlet temperature and rate of charging on the maximum bed temperature and the time required to fill the cylinder. (C) 2004 Elsevier Ltd. All rights reserved.
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