Journal
JOURNAL OF PORPHYRINS AND PHTHALOCYANINES
Volume 11, Issue 5-6, Pages 463-469Publisher
WORLD SCI PUBL CO INC
DOI: 10.1142/S1088424607000539
Keywords
Cu(III) corrole; [Ru(bpy)(3)](2+); OEC; photosystem II; water oxidation
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A novel binuclear Ru-Cu complex, composed of a copper(III)-corrole and a ruthenium(II) tris(bipyridine) moicty linked by an amide bond, has been synthesized and characterized by H-1 NMR, UV-vis and mass spectrometry. The steady-state emission and the electrochemical properties were investigated. Compared to the parent [Ru(bpy)(3)](2+), the emission-of the desired complex was substantially quenched when the MLCT of [Ru(bpy)(3)](2+) was selectively photoexcited. Copyright (C) 2007. Society of Porphyrins & Phthalocyanines.
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