Journal
RESEARCH ON CHEMICAL INTERMEDIATES
Volume 33, Issue 3-5, Pages 239-250Publisher
VSP BV
DOI: 10.1163/156856707779238667
Keywords
oxygen isotopic exchange; semiconductor; calcination; titanium dioxide catalyst; photocatalysis
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This article first indicates the various types of temperature-induced oxygen isotopic exchange (OIE) that can occur between labeled gaseous O-2 and solid oxides. Earlier main results of light-induced OIE with semiconductor oxides are then briefly reviewed. The core of the article reports new results about the use of light-induced OIE to assess (i) the lability of TiO2 surface O atoms, as altered by calcination or Se deposits, via the comparison of OIE with the photocatalytic removal of methanol in air and (ii) the accessibility of TiO2 affixed on a fiberglass material by means of a silica binder. Both this overview and these novel results illustrate the interest of OIE in heterogeneous photocatalysis.
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