Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 13, Issue 13, Pages 3804-3812Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.200601561
Keywords
charge transfer; donor-acceptor systems; nitrogen heterocycles; photophysical properties; tetrathiafulvalene
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To study the electronic interactions in donor-acceptor (D-A) ensembles, D and A fragments are coupled in a single molecule. Specifically, a tetrathiafulvalene (TTF)-fused dipyrido[3,2-a:2',3'-c]phenazine (dppz) compound having inherent redox centers has been synthesized and structurally characterized. Its electronic absorption, fluorescence emission, photoinduced intramolecular charge transfer, and electrochemical behavior have been investigated. The observed electronic properties are explained on the basis of density functional theory.
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