Journal
JOURNAL OF THE EUROPEAN CERAMIC SOCIETY
Volume 27, Issue 16, Pages 4767-4772Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.jeurceramsoc.2007.04.004
Keywords
Si2N2O; sintering; mechanical properties; dielectric properties
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Dense Si2N2O was successfully synthesized using 2 mol% Li2O as an additive by a hot-pressing method at 1500 degrees C. Compared to other metal oxide additives, Li2O can significantly decrease the sintering temperature of Si2N2O, which is ascribed to the lower melting point of Li2O-SiO2 and the formation of less viscous liquid phase. Increasing Li2O content has no apparent influence on the mechanical and dielectric properties of dense Si2N2O, which is due to the easy evaporation of Li2O at sintering temperature. The mechanical properties of Si2N2O with Li2O additive are comparable to those of Si2N2O synthesized with other additives. The as-prepared bulk Si2N2O with 2 mol% Li2O additive exhibits both low dielectric constant (6.17 at 1 MHz) and loss tangent (0.0008 at 1 MHz) and combines good mechanical performance, indicating it is a potential high-temperature structural/functional material. (C) 2007 Elsevier Ltd. All rights reserved.
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