Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 13, Issue 33, Pages 9216-9222Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.200700860
Keywords
cyclodextrins; fluorescence; hydrosol-gel; photoisomerization; reversible systems; rotaxanes
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Rotaxane-based nanoscale architectures have a huge potential to be processed into widely applied devices. In this work, light-driven rotaxanes with fluorescent chromophores based on a-cyclodextrin (alpha-CyD) have been doped into amphoteric thermoreversible hydrosol-gels to form a new type of disperse system with reversible optical signals. The photoisomerizations with alpha-CyD shuttling have been studied by induced circular dichroism (ICD). Compared with their corresponding solutions, the rotaxane-doped hydrosol-gel systems produce much more obvious fluorescent binary signals.
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