☆ 4.5 Article

Copper-catalyzed transformation of carbonyl-ene-nitrile compounds: Vinylation, imino ene reaction, and alkynylation of 2-aza-2,4-cyclopentadienone intermediates generated via Ritter-type hydratrion and dehydrative cyclization reactions

JOURNAL OF ORGANOMETALLIC CHEMISTRY (2007)

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Journal

JOURNAL OF ORGANOMETALLIC CHEMISTRY
Volume 692, Issue 1-3, Pages 579-584

Publisher

ELSEVIER SCIENCE SA
DOI: 10.1016/j.jorganchem.2006.04.053

Keywords

copper(II)-catalysis; carbonyl-ene-nitrile; azacyclopentadienone; pyrrolinone; vinylation; allylation

Categories

Chemistry, Inorganic & Nuclear Chemistry, Organic

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1H-pyrrolin-2(5H)-one derivatives are easily obtained from carbonyl-ene-nitrile compounds and alkenes or alklynes by copper(II)-catalyzed tandem sequence involving vinylation or allylation as well as Ritter-type hydration and dehydrative cyclization. (c) 2006 Elsevier B.V. All rights reserved.

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